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Chemisorption solid materials for hydrogen storage near ambient temperature: a review

Yiheng ZHANG, Shaofei WU, Liwei WANG, Xuefeng ZHANG

《能源前沿（英文）》 2023年 第17卷 第1期   页码 72-101 doi: 10.1007/s11708-022-0835-7

摘要： Solid chemisorption technologies for hydrogen storage, especially high-efficiency hydrogen storage of fuel cells in near ambient temperature zone defined from −20 to 100°C, have a great application potential for realizing the global goal of carbon dioxide emission reduction and vision of carbon neutrality. However, there are several challenges to be solved at near ambient temperature, i.e., unclear hydrogen storage mechanism, low sorption capacity, poor sorption kinetics, and complicated synthetic procedures. In this review, the characteristics and modification methods of chemisorption hydrogen storage materials at near ambient temperature are discussed. The interaction between hydrogen and materials is analyzed, including the microscopic, thermodynamic, and mechanical properties. Based on the classification of hydrogen storage metals, the operation temperature zone and temperature shifting methods are discussed. A series of modification and reprocessing methods are summarized, including preparation, synthesis, simulation, and experimental analysis. Finally, perspectives on advanced solid chemisorption materials promising for efficient and scalable hydrogen storage systems are provided.

关键词： hydrogen storage capacity     chemisorption     near-ambient-temperature     modification methods     alloy hydrides    

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Evaluating the short-term effect of ambient temperature on non-fatal outdoor falls and road traffic injuries

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1705-1

摘要：

● A study assessing the temperature-injury relationship was conducted among students.

关键词： Ambient temperature     Fall     Road traffic injury     Student     China    

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Prediction of the theoretical and semi-empirical model of ambient temperature

Foued CHABANE,Noureddine MOUMMI,Abdelhafid BRIMA,Abdelhafid MOUMMI

《能源前沿（英文）》 2016年 第10卷 第3期   页码 268-276 doi: 10.1007/s11708-016-0413-y

摘要： It is well known that the ambient temperature is a sensitive parameter which has a great effect on biology, technology, geology and even on human behavior. A prediction is a statement about an uncertain event. It is often, but not always, based upon experience or knowledge. Although guaranteed accurate information about the future is in many cases impossible, prediction can be useful to assist in making plans about possible developments. As a result, temperature profiles can be developed which accurately represent the expected ambient temperature exposure that this environment experiences during measurement. The ambient temperature over time is modeled based on the previous and data and using a Lagrange interpolation. To observe the comprehensive variation of ambient temperature the profile must be determined numerically. The model proposed in this paper can provide an acceptable way to measure the change in ambient temperature.

关键词： ambient temperature     environment     correlation     theoretical model     semi-empirical    

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Effects of ambient temperature on regulated gaseous and particulate emissions from gasoline-, E10- and

Rencheng Zhu, Jingnan Hu, Liqiang He, Lei Zu, Xiaofeng Bao, Yitu Lai, Sheng Su

《环境科学与工程前沿（英文）》 2021年 第15卷 第1期 doi: 10.1007/s11783-020-1306-1

摘要： Abstract • Emissions from two sedans were tested with gasoline, E10 and M15 at 30°C and -7°C. • As the temperature decreased, the PM, PN and BC emissions increased with all fuels. • Particulate emissions with E10 and M15 were more sensitive to the temperature. • The PN and BC generated during cold start-up dominated those over the WLTC. Ambient temperature has substantial impacts on vehicle emissions, but the impacts may differ between traditional and alcohol gasolines. The objective of this study was to investigate the effects of temperature on gaseous and particulate emissions with both traditional and alcohol gasoline. Regulated gaseous, particle mass (PM), particle number (PN) and black carbon (BC) emissions from typical passenger vehicles were separately quantified with gasoline, E10 (10% ethanol and 90% gasoline by volume) and M15 (15% methanol and 85% gasoline by volume) at both 30°C and -7°C. The particulate emissions with all fuels increased significantly with decreased temperature. The PM emissions with E10 were only 48.0%–50.7% of those with gasoline at 30°C but increased to 59.2%-79.4% at -7°C. The PM emissions with M15 were comparable to those with gasoline at 30°C, but at -7°C, the average PM emissions were higher than those with gasoline. The variation trend of PN emissions was similar to that of PM emissions with changes in the fuel and temperature. At 30°C, the BC emissions were lower with E10 and M15 than with gasoline in most cases, but E10 and M15 might emit more BC than gasoline at -7°C, especially M15. The results of the transient PN and BC emission rates show that particulate emissions were dominated mainly by those emitted during the cold-start moment. Overall, the particulate emissions with E10 and M15 were more easily affected by ambient temperature, and the advantages of E10 and M15 in controlling particulate emissions declined as the ambient temperature decreased.

关键词： Particle mass     Particle number     Black carbon     Alcohol gasoline     Low temperature    

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Numerical investigation on side heat transfer enhancement in 300 kA aluminum reduction cell

WANG Changhong, ZHU Dongsheng, LEI Junxi, ZHOU Jiemin

《能源前沿（英文）》 2008年 第2卷 第3期   页码 256-260 doi: 10.1007/s11708-008-0051-0

摘要： Industrial test and numerical simulation were synchronously applied to analyze the side heat transfer process and enhance heat transfer in aluminum reduction cell. The 3D slice finite element model of aluminum reduction cell was developed, with which the sidewall temperature field of the cell was computed by using software ANSYS. The main influencing factors on heat dissipation were analyzed and some effective measures were proposed to enhance sidewall heat transfer. The results show that the shell temperature of the test cell and the common cell is respectively 312°C and 318°C and the ledge thickness is 16 cm and 15 cm when side coefficient of heat transfer between the shell and the surroundings is 70 W/(mK). With the increase of the side coefficient of heat transfer between the shell and the surroundings, the temperature of the shell decreases but the thickness of the side ledge increases when the electrolytic temperature, the ambient temperature, the coefficient of heat transfer between molten bath and ledge, the eutectic temperature and the thermo-resistance of the side lining are constant.

关键词： constant     ambient temperature     thickness     electrolytic temperature     transfer process    

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Correlations for estimating solar radiation using sunshine hours and temperature measurement in Osogbo

O. S. OHUNAKIN, M. S. ADARAMOLA, O. M. OYEWOLA, R. O. FAGBENLE

《能源前沿（英文）》 2013年 第7卷 第2期   页码 214-222 doi: 10.1007/s11708-013-0241-2

摘要： In this study, the global solar radiation on horizontal surface in Osogbo, Osun state, Nigeria was analyzed using 11-year data (1997–2007). Correlations using linear and quadratic expressions were developed to relate the global solar radiation on horizontal surface based on relative sunshine hours and temperature measurements for evaluating the monthly average daily global solar radiation. The calculated monthly clearness index values indicate that the prevailing weather condition in Osogbo is heavily overcast. All the developed quadratic correlations gave better correlation coefficients (0.834, 0.872 and 0.823 respectively) than the linear models. However, the Hargreaves and Samani related based quadratic model gave the best among the three developed quadratic expressions and is therefore suggested for estimating the monthly global radiation in this site and its surroundings.

关键词： global solar radiation     Hargreaves model     sunshine hour     ambient temperatures     Osogbo    

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Human health ambient water quality criteria for 13 heavy metals and health risk assessment in Taihu Lake

《环境科学与工程前沿（英文）》 2022年 第16卷 第4期 doi: 10.1007/s11783-021-1475-6

摘要：

• The concentrations of 13 heavy metals in Taihu Lake were analyzed.

关键词： Heavy metals     Human health ambient water quality criteria     Taihu Lake     Health risk assessment     Contribution rate    

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Hygroscopicity of ambient submicron particles in urban Hangzhou, China

Jiachen ZHANG, Lin WANG, Jianmin CHEN, Shengmao FENG, Jiandong SHEN, Li JIAO

《环境科学与工程前沿（英文）》 2011年 第5卷 第3期   页码 342-347 doi: 10.1007/s11783-011-0358-7

摘要： In this study, hygroscopicity of size-segregated ambient submicron particles in urban Hangzhou was studied from 28th December 2009 to 18th January 2010, using a hygroscopicity-tandem differential mobility analyzer (H-TDMA). The submicron particles in Hangzhou showed a minor hygroscopic growth at 73% relative humidity (RH), and then grew significantly between 77% and 82% RH. Monomodal distribution accounted for 90% for 30 nm particles, 17% for 50 nm particles, and less than 7% for particles larger than 50 nm at 82% RH. Deconvolution of the bimodal distribution indicated a less hygroscopic group and a more hygroscopic group, with the fraction of the more hygroscopic group increasing with the initial dry particle size and then remaining almost constant for accumulation mode particles. Our results imply that submicron particles in urban Hangzhou were almost entirely externally mixed, and the hygroscopic properties of ambient particles in urban Hangzhou were mainly a function of their size and chemical composition.

关键词： hygroscopicity     hygroscopic tandem differential mobility analyzer (H-TDMA)     submicron ambient particles     Hangzhou    

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Effect of ambient polycyclic aromatic hydrocarbons and nicotine on the structure of Aβ protein

《环境科学与工程前沿（英文）》 2023年 第17卷 第2期 doi: 10.1007/s11783-023-1615-2

摘要：

● B[a]P, nicotine and phenanthrene molecules altered the secondary structure of Aβ42.

关键词： Polycyclic aromatic hydrocarbons     Nicotine     toxicology     Aβ42 peptide     Alzheimer’s disease     Molecular dynamics simulations     Environmental pollution    

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Effect of sodium bicarbonate solution on methyltrimethoxysilane-derived silica aerogels dried at ambient

Yujing Liu, Xiao Han, Balati Kuerbanjiang, Vlado K. Lazarov, Lidija Šiller

《化学科学与工程前沿（英文）》 2021年 第15卷 第4期   页码 954-959 doi: 10.1007/s11705-020-2028-4

摘要： Here we present an economical ambient pressure drying method of preparing monolithic silica aerogels from methyltrimethoxysilane precursor while using sodium bicarbonate solution as the exchanging solvent. We prepared silica aerogels with a density and a specific surface area of 0.053 g∙cm and 423 m ∙g , respectively. The average pore diameter of silica aerogels is 23 nm as the pore specific volume is 1.11 cm ∙g . Further, the contact angle between water droplet and the surface of silica aerogels in specific condition can be as high as 166°, which indicates a super-hydrophobic surface of aerogels.

关键词： silica aerogel     methyltrimethoxysilane     solvent exchange     sodium bicarbonate     trimethylchlorosilane     ambient pressure drying    

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珊瑚岛礁环境噪声成像 Article

夏少红, 张昌榕, 曹敬贺

《工程（英文）》 2023年 第25卷 第6期   页码 182-193 doi: 10.1016/j.eng.2021.09.022

摘要：

As valuable land in the ocean, coral islands are not only important bases for making use of marine resources and protecting marine rights and interests, but also important for breakthrough research in many fields of earth science. Hence, the economical and efficient determination of the underground structure of coral islands has become significant in coral island engineering geology, but remains challenging for traditional marine geophysical prospecting and drilling methods. While ambient noise tomography with dense arrays has been widely used in continental regions, its applicability to coral islands remains undetermined. In this study, based on the data recorded by a dense array on an isolated coral island in the South China Sea, we analyzed the ambient noise characteristics and obtained a 3D subsurface structure of the coral island using ambient noise tomography. We made the following findings: ① The ambient noise frequencies can be roughly categorized into three levels: < 1, 1–5, and > 5 Hz. The spectral characteristics of the noise below 5 Hz were consistent at different stations, but there were significant differences in the characteristics of the noise above 5 Hz. ② For ambient noise frequencies below 5 Hz, cross-correlation functions with high quality could be obtained with only 24 h of waveform data. However, it was difficult to extract meaningful cross-correlation functions for ambient noise frequencies above 5 Hz. ③ The S-wave velocity in the coral island was higher toward the sea and lower toward the lagoon, which was consistent with the high degree of cementation of the outer reef flat stratum on the seaward side. ④ There were two low-velocity horizons at 25–75 and 200–300 m, which were in good agreement with the high-porosity horizons that were revealed by drilling core samples, reflecting the weathering history of the reef. Our research demonstrates that ambient noise tomography is a potentially economical, efficient, and environmentally friendly method for the geological prospecting of coral reefs.

关键词： Coral island     Ambient noise tomography     Engineering geology     South China Sea    

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Hybrid energy harvesting systems for self-powered sustainable water purification by harnessing ambient

《环境科学与工程前沿（英文）》 2023年 第17卷 第10期 doi: 10.1007/s11783-023-1718-9

摘要：

● Energy harvesters harness multiple energies for self-powered water purification.

关键词： Piezocatalysis     Solar energy     Waste heat     Decentralized water treatment     Point-of-use     Nanogenerator    

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Experimental study of modal parameter identification in a simulated ambient-excited structure

JI Xiaodong, QIAN Jiaru, XU Longhe

《结构与土木工程前沿（英文）》 2007年 第1卷 第3期   页码 281-285 doi: 10.1007/s11709-007-0036-9

摘要： Structure modal parameter online identification was used to monitor the structural health as evidenced by changes in the vibration characteristics. The natural excitation technique and the eigensystem realization algorithm were combined to identify the modal parameters in the time domain of a structure excited by simulated ambient vibrations. The mass-normalized mode shapes were obtained from the eigen-sensitivity analysis. The experimental modal analysis was performed on a two-story steel braced frame model excited by simulated ambient vibrations and hammer impacts. The mass-normalized mode shapes were acquired by changing the structural mass and by eigen-sensitivity analy sis. From finite element analysis results and the experimental data, it is shown that this method is effective.

关键词： eigensystem realization     eigen-sensitivity analysis     realization algorithm     vibration     effective    

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综合空气污染和非适宜温度相关死亡风险构建空气健康指数 Article

张庆丽, 陈仁杰, 印冠锦, 杜喜浩, 孟夏, 邱杨, 阚海东, 周脉耕

《工程（英文）》 2022年 第14卷 第7期   页码 156-162 doi: 10.1016/j.eng.2021.05.006

摘要：

综合的空气健康指数有助于强调多种大气危险因素的健康风险，有利于向公众传达不良大气环境的总体风险。本文试图通过整合我国大气污染和非适宜温度相关的每日死亡风险，建立一种新的空气健康指数（Air Health Index, AHI）。本研究从时间序列模型中获得了暴露-反应系数，通过将 2013—2015 年我国 272个城市大气污染物与非适宜温度相关的超额死亡风险求和，构建了新的AHI。估计了基于总死亡率构建的AHI（“总AHI”）与全死因死亡率的关系，并进一步比较了“总AHI”与“特异性AHI”（基于疾病别死 亡率构建）在预测心肺系统疾病死亡率方面的能力。研究发现，空气污染和非适宜温度与28.23%的每日超额死亡率有关，其中23.47%与非适宜温度有关，其余的与PM2.5（1.12%）、NO2（2.29%）和O3（ 2.29%）有关。新的AHI采用了10分制的评分标准，272座城市的平均AHI为6分。AHI与死亡率关系的暴露-反应曲线呈线性，不存在阈值。“总AHI”每增加一个单位，全死因死亡率增加0.84%，心血管疾病、冠心病、中风、呼吸系统疾病和慢性阻塞性肺疾病的死亡率分别增加1.01%、0.98%、1.02%、1.66%和1.71%。使用“总AHI”估计疾病别死亡率风险与使用“特异性AHI”预测的疾病别死亡率风险相似。综上所述，本研究提出的“总AHI”可能是一种有前途的风险交流工具，有利于向公众传达与大气环境有关的健康风险。

关键词： 大气污染     温度     空气健康指数     死亡     时间序列     风险交流    

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iterative data enhancement for implementation in purification of modal frequency for extremely noisy ambient

Hassan YOUSEFI, Alireza TAGHAVI KANI, Iradj MAHMOUDZADEH KANI, Soheil MOHAMMADI

《结构与土木工程前沿（英文）》 2020年 第14卷 第2期   页码 446-472 doi: 10.1007/s11709-019-0605-8

摘要： The main purpose of the present study is to enhance high-level noisy data by a wavelet-based iterative filtering algorithm for identification of natural frequencies during ambient wind vibrational tests on a petrochemical process tower. Most of denoising methods fail to filter such noise properly. Both the signal-to-noise ratio and the peak signal-to-noise ratio are small. Multiresolution-based one-step and variational-based filtering methods fail to denoise properly with thresholds obtained by theoretical or empirical method. Due to the fact that it is impossible to completely denoise such high-level noisy data, the enhancing approach is used to improve the data quality, which is the main novelty from the application point of view here. For this iterative method, a simple computational approach is proposed to estimate the dynamic threshold values. Hence, different thresholds can be obtained for different recorded signals in one ambient test. This is in contrast to commonly used approaches recommending one global threshold estimated mainly by an empirical method. After the enhancements, modal frequencies are directly detected by the cross wavelet transform (XWT), the spectral power density and autocorrelation of wavelet coefficients. Estimated frequencies are then compared with those of an undamaged-model, simulated by the finite element method.

关键词： ambient vibration test     high level noise     iterative signal enhancement     wavelet     cross and autocorrelation of wavelets    

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标题 作者 时间 类型 操作

Chemisorption solid materials for hydrogen storage near ambient temperature: a review

Yiheng ZHANG, Shaofei WU, Liwei WANG, Xuefeng ZHANG

期刊论文

Evaluating the short-term effect of ambient temperature on non-fatal outdoor falls and road traffic injuries

期刊论文

Prediction of the theoretical and semi-empirical model of ambient temperature

Foued CHABANE,Noureddine MOUMMI,Abdelhafid BRIMA,Abdelhafid MOUMMI

期刊论文

Effects of ambient temperature on regulated gaseous and particulate emissions from gasoline-, E10- and

Rencheng Zhu, Jingnan Hu, Liqiang He, Lei Zu, Xiaofeng Bao, Yitu Lai, Sheng Su

期刊论文

Numerical investigation on side heat transfer enhancement in 300 kA aluminum reduction cell

WANG Changhong, ZHU Dongsheng, LEI Junxi, ZHOU Jiemin

期刊论文

Correlations for estimating solar radiation using sunshine hours and temperature measurement in Osogbo

O. S. OHUNAKIN, M. S. ADARAMOLA, O. M. OYEWOLA, R. O. FAGBENLE

期刊论文

Human health ambient water quality criteria for 13 heavy metals and health risk assessment in Taihu Lake

期刊论文

Hygroscopicity of ambient submicron particles in urban Hangzhou, China

Jiachen ZHANG, Lin WANG, Jianmin CHEN, Shengmao FENG, Jiandong SHEN, Li JIAO

期刊论文

Effect of ambient polycyclic aromatic hydrocarbons and nicotine on the structure of Aβ protein

期刊论文

Effect of sodium bicarbonate solution on methyltrimethoxysilane-derived silica aerogels dried at ambient

Yujing Liu, Xiao Han, Balati Kuerbanjiang, Vlado K. Lazarov, Lidija Šiller

期刊论文

珊瑚岛礁环境噪声成像

夏少红, 张昌榕, 曹敬贺

期刊论文

Hybrid energy harvesting systems for self-powered sustainable water purification by harnessing ambient

期刊论文

Experimental study of modal parameter identification in a simulated ambient-excited structure

JI Xiaodong, QIAN Jiaru, XU Longhe

期刊论文

综合空气污染和非适宜温度相关死亡风险构建空气健康指数

张庆丽, 陈仁杰, 印冠锦, 杜喜浩, 孟夏, 邱杨, 阚海东, 周脉耕

期刊论文

iterative data enhancement for implementation in purification of modal frequency for extremely noisy ambient

Hassan YOUSEFI, Alireza TAGHAVI KANI, Iradj MAHMOUDZADEH KANI, Soheil MOHAMMADI

期刊论文